In the Valley of Ashes, kill 100 Asherisen Captains, then report to Ashen Bones.

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Introduction

Ashen Bones has asked you to kill Asherisen Captains so that it can recover its magic.

NPC Dialog

I take no pleasure in the sight of death, but the souls of my enemies are the only way for me to recover my magic. Those Asherisen Captains stole my master's ashes and scattered them across the valley. Evil creatures like that deserve no mercy.

Quest Completion

It pains me do ask this of you, but this is the only method there is to recover my magic...